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Journal Articles

Automation of precise gas control for material-process researches; Application to synchrotron radiation real-time observation of surface reactions

Nakamura, Takafumi*; Yamamoto, Yukio*; Arakawa, Masakazu*; Maruyama, Akio*; Yoshigoe, Akitaka

Sangyo Oyo Kogakukai Rombunshi, 11(2), p.109 - 114, 2023/09

Surface chemistry experimental end-station at BL23SU in SPring-8 is widely used to study various surfaces and interfaces of functional materials by means of soft X-rays synchrotron radiation. To analyze surface chemical reactions between gas and solid surfaces, an accurate control of flow-rates of gases is essential. This paper describes a computerized automatic gas flow control system to improve the accuracy and reproducibility of gas-surface reaction experiments in the pressure range of ultra-high vacuum (molecular flow) conditions. The system uses feedback control to operate the slow-leak valve to control the gas-pressure. As a result, the system achieved results equivalent to those of a skilled experimenter.

Journal Articles

Novel hydrogel properties by microstructural control of carboxymethyl cellulose nanofibers using freezing

Sekine, Yurina

Fain Kemikaru, 52(8), p.25 - 32, 2023/08

By using the freezing phenomenon, we discovered that a hydrogel with high compressive strength can be formed using only harmless materials, mainly carboxymethyl cellulose nanofibers. The key is the phase separation of ice crystals and solutes that occurs when aqueous solutions freeze. This paper describes the formation mechanism of the freeze crosslinked hydrogel and its properties.

Journal Articles

Probing copper and copper-gold alloy surfaces with space-quantized oxygen molecular beam

Tsuda, Yasutaka; Gueriba, J. S.*; Ueta, Hirokazu*; Di$~n$o, W. A.*; Kurahashi, Mitsunori*; Okada, Michio*

JACS Au (Internet), 2(8), p.1839 - 1847, 2022/08

Journal Articles

Status of LBE study and experimental plan at JAEA

Saito, Shigeru; Wan, T.*; Okubo, Nariaki; Obayashi, Hironari; Watanabe, Nao; Ohdaira, Naoya*; Kinoshita, Hidetaka; Yamaki, Kenichi*; Kita, Satoshi*; Yoshimoto, Hidemitsu*; et al.

JPS Conference Proceedings (Internet), 33, p.011041_1 - 011041_6, 2021/03

An Accelerator Driven System (ADS) for waste transmutation investigated in JAEA employs lead-bismuth eutectic (LBE) as a neutron production target material and coolant. The neutrons are to be produced via the spallation with 1.5 GeV proton beam injection. As materials irradiation data are important for ADS development, JAEA plans to construct an irradiation facility with LBE neutron production target in J-PARC. There are many technical issues on LBE for practical use. In JAEA, various R&Ds are being carried out. Concerning corrosion study, conditioning operation and functional tests of OLLOCHI started. Oxygen concentration control technology has also developing. In the large scale LBE loop experiment, the operation for steady state and transient experiments was performed by using IMMORTAL. In the area of instrument, development of ultrasonic flow meter and freeze seal valve are progressing as a key technology for the LBE loop system. Investigation of behavior of impurities in LBE, which is important for design of the irradiation facility, started. In this paper, the status of the LBE studies and experimental plan will be presented.

Journal Articles

250 kW LBE spallation target for ADS development in J-PARC

Sasa, Toshinobu; Saito, Shigeru; Obayashi, Hironari; Ariyoshi, Gen

JPS Conference Proceedings (Internet), 33, p.011051_1 - 011051_6, 2021/03

To realize Accelerator-driven system (ADS) for minor actinide transmutation, JAEA proposes to construct the Proton Irradiation Facility in J-PARC. The facility is planned to solve technical issues for safe application of Lead-bismuth Eutectic Alloy (LBE). The 250 kW LBE spallation target will be located in the facility to prepare material irradiation database by both proton and neutron irradiation in the temperature range for typical LBE-cooled ADS. Various studies for important technologies required to build the facilities are investigated such as oxygen concentration control, instruments development, remote handling techniques for target maintenance, and spallation target design. The large scale LBE loops for mock up the 250 kW LBE spallation target and material corrosion studies are also manufactured and applied to various experiments. The latest status of 250 kW LBE spallation target design works will be summarized.

Journal Articles

Electric current control of spin helicity in an itinerant helimagnet

Jiang, N.*; Nii, Yoichi*; Arisawa, Hiroki*; Saito, Eiji; Onose, Yoshinori*

Nature Communications (Internet), 11, p.1601_1 - 1601_6, 2020/03

 Times Cited Count:28 Percentile:85.73(Multidisciplinary Sciences)

Journal Articles

Study on fracture behaviour of through-wall cracked elbow under displacement control load

Machida, Hideo*; Koizumi, Yu*; Wakai, Takashi; Takahashi, Koji*

Nihon Kikai Gakkai M&M 2019 Zairyo Rikigaku Kanfarensu Koen Rombunshu (Internet), p.OS1307_1 - OS1307_5, 2019/11

This paper describes the fracture test and fracture analysis of a pipe under displacement control load. In order to grasp the fracture behavior of the circumferential through-wall cracked pipe, which is important in evaluating the feasibility of leak before break (LBB) in sodium cooled reactor piping, a fracture test in case of a circumferential throughwall crack in the weld line between an elbow and a straight pipe was carried out. From this test, it was found that no pipe fracture occurs in the displacement control loading condition even if a large circumferential through-wall crack (180$$^{circ}$$) was assumed. The fracture analysis of the pipe was carried out using Gurson's parameters set based on the tensile test results of the tested pipe material. The analytic results agree well with the test results, and it was found that it will be possible to predict the fracture behavior of sodium cooled reactor piping.

Journal Articles

Laser cutting technology of thick steel components; Advanced technology developed at the era of decommissioning

Tamura, Koji*; Toyama, Shinichi

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 61(5), p.413 - 415, 2019/05

In decommissioning of nuclear reactors, it is necessary to disassemble the nuclear reactor structure. In addition to the conventional cutting method, the laser method has many advantages such as remote controllability and no need for replacement parts such as blades, which can be a powerful choice. Nuclear reactor structure such as a pressure vessel are made of steel materials with a thickness exceeding 100 mm, and the laser method has poor knowledge and experience in cutting such thick steel materials. Therefore, as a result of trial cutting of steel materials under various cutting conditions with the high power fiber laser which is progressively available nowadays, it has been demonstrated that laser cutting is also possible for thick plates such as those used in nuclear reactors, and cutting of thick steel plates. We also developed the cutting technology using remote control using a robot in order to apply it to the decommissioning of thick steel cutting on the spot.

Journal Articles

Holding force tests of Curie Point Electro-Magnet in hot gas for passive shutdown system

Matsunaga, Shoko*; Matsubara, Shinichiro*; Kato, Atsushi; Yamano, Hidemasa; D$"o$derlein, C.*; Guillemin, E.*; Hirn, J.*

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05

This paper presents a design of Curie Point Electro-Magnet (CPEM) which will be installed as a passive shutdown system for a French Sodium-cooled Fast Reactor (ASTRID) development program which is conducted in collaboration between France and Japan. To confirm CPEM design validity, a qualification program for CPEM is developed on the basis of past comprehensive test series of Self-Actuated Shutdown System (SASS) in Japan. The main outcome of this paper is results of holding force tests in hot gas, which satisfy design requirements. Moreover, the result of a numerical magnetic field analysis showed the same tendency as that of the holding force test.

Journal Articles

Quantum optimal control of rovibrational excitations of a diatomic alkali halide; One-photon vs. two-photon processes

Kurosaki, Yuzuru*; Yokoyama, Keiichi

Universe (Internet), 5(5), p.109_1 - 109_15, 2019/05

 Times Cited Count:0 Percentile:0.01(Astronomy & Astrophysics)

Regarding rovibrational transitions of diatomic alkali haride molecules, optimal waveform of laser electric field was calculated on the basis of the optimal control theory. In this study, we implemented the polarizability term into the Hamiltonian, which defines the field-molecule interaction. As a result, we obtained waveforms causing both one- and two-photon processes in a relatively high electric field regime, while waveforms causing only one-photon process was observed in a weak filed regime as well as the previous study. These results imply that the effect of two-photon process is successfully taken into account in the optimal control theory calculation. Now we can expect more reliable calculation even for strong laser field.

Journal Articles

Development of synthesis and morphology control method of metallic oxide particles using microwave heating

Segawa, Tomoomi

Funtai Kogakkai-Shi, 55(10), P. 547, 2018/10

no abstracts in English

Journal Articles

Physical and electrical characterizations of AlGaN/GaN MOS gate stacks with AlGaN surface oxidation treatment

Yamada, Takahiro*; Watanabe, Kenta*; Nozaki, Mikito*; Shih, H.-A.*; Nakazawa, Satoshi*; Anda, Yoshiharu*; Ueda, Tetsuzo*; Yoshigoe, Akitaka; Hosoi, Takuji*; Shimura, Takayoshi*; et al.

Japanese Journal of Applied Physics, 57(6S3), p.06KA07_1 - 06KA07_6, 2018/06

 Times Cited Count:6 Percentile:30.01(Physics, Applied)

Thermal oxidation of AlGaN surface and its impact on the electrical properties of AlGaN/GaN MOS capacitors were investigated by means of synchrotron radiation photoelectron spectroscopy (SR-PES), atomic force microscopy (AFM) and C-V measurements. SR-PES analysis revealed that the AlGaN surface is oxidized even at low temperature of 400$$^{circ}$$C, in contrast to no oxide formation on GaN surface. However, since no noticeable change in the surface morphology was observed at temperatures up to 800$$^{circ}$$C, it can be concluded that an ultrathin oxide overlayer is formed on the AlGaN surface. On the other hand, for the oxidation treatments above 850$$^{circ}$$C, the formation of small oxide grains was observed over the entire area of the AlGaN surface, and the growth of oxide grains significantly degraded the surface morphology. Therefore, the AlGaN/GaN MOS capacitors were fabricated on the AlGaN surface oxidized at moderate temperatures up to 800$$^{circ}$$C. While we have confirmed that relatively good interface properties are obtained for direct AlON deposition without oxidation treatment, it was found that the oxidation treatment at 400$$^{circ}$$C leads to further improvement of interface properties and reduction of C-V hysteresis.

Journal Articles

Research on nanostructure-controlled functional membranes using high-energy ion beams; Fluoropolymer-based porous and ion-exchange membranes

Yamaki, Tetsuya*; Kitamura, Akane; Sawada, Shinichi*; Koshikawa, Hiroshi*

Nihon Kaisui Gakkai-Shi, 72(2), p.62 - 74, 2018/04

This review paper is devoted to two topics, i.e., fluoropolymer-based porous and ion-exchange membranes, both of which include the creation of nanostructure-controlled functional membranes with high-energy ion beams. Latent tracks of the MeV-GeV heavy ions in a polymer foil can sometimes be chemically etched out to form a membrane with micro- and nano-sized through-pores, the so-called ion-track membrane. Our focus is on ion-track membranes of poly (vinylidene fluoride) (PVDF) and cation- and anion-exchange membranes (CEMs and AEMs, respectively).

Journal Articles

Phenomenology of BWR fuel assembly degradation

Kurata, Masaki; Barrachin, M.*; Haste, T.*; Steinbrueck, M.*

Journal of Nuclear Materials, 500, p.119 - 140, 2018/03

 Times Cited Count:29 Percentile:66.35(Materials Science, Multidisciplinary)

Severe accidents occurred at the Fukushima-Daiichi Nuclear Power Station (FDNPS) required an immediate re-examination of fuel degradation phenomenology. The present paper reviews the updated knowledge on the phenomenology of the fuel degradation, focusing mainly on the BWR fuel assembly degradation at the macroscopic scale and that of the individual interactions at the meso-scale. Oxidation of boron carbide (B$$_{4}$$C) control rods potentially generate far larger amounts of heat and hydrogen under BWR accident conditions. All integral tests with B$$_{4}$$C control rods or control blades have shown early failure, liquefaction, relocation and oxidation of B$$_{4}$$C starting at temperatures around 1250$$^{circ}$$C, well below the significant interaction temperatures of UO$$_{2}$$-Zry. These interactions or reactions potentially influence the progress of fuel degradation in the early phase. The steam-starved conditions, which are being discussed as a likely scenario at the FDNPS accident, highly influence the individual interactions and potentially lead the fuel degradation in non-prototypical directions. The detailed phenomenology of individual interactions and their influence on the transient and on the late phase of the severe accidents are also discussed.

Journal Articles

Micro-orientation control of silicon polymer thin films on graphite surfaces modified by heteroatom doping

Shimoyama, Iwao; Baba, Yuji; Hirao, Norie*

Advances in Engineering (Internet), 1 Pages, 2018/02

The performance of organic devices largely depends on molecular orientation in organic films. Whereas micro-orientation control of organic molecules is an indispensable technology for integration of organic devices, the method has not been established. We attempted to control micro-orientation of polydimethylsilane (PDMS) thin films by deposition of PDMS on graphite substrates modified by hetero atom doping using ion beam. Polarization dependence measurements of X-ray absorption spectroscopy and molecular orbital calculations clarified that PDMS films have lying, standing, and random orientations on the non irradiated, N$$_{2}$$$$^{+}$$-irradiated, and Ar$$^{+}$$-irradiated graphite surfaces, respectively. Furthermore, photoemission microscopy observation clarified that a PDMS film showed micro-patterns on a graphite surface with a microstructure on the order of $$mu$$m by separating N$$_{2}$$$$^{+}$$-irradiated and non irradiated areas. These results demonstrate our method is promising for micro-orientation of organic molecules.

Journal Articles

Development of an altitude-keeping system for underwater robots using laser beams

Takemura, Fumiaki*; Taba, Ryo*; Hirayama, Keita*; Tansuriyavong, S.*; Kawabata, Kuniaki; Sagara, Shinichi*; Ogasawara, Kei*

Artificial Life and Robotics, 22(4), p.405 - 411, 2017/12

The manta method is a survey method that divers investigate the degree of coral and whitening state while being towed to a boat. The manta method makes great physical burden. Therefore, the authors think that this task can substitute an underwater robot. This underwater robot is desirable to be able to keep altitude above the seabed. Hence, the authors have been developing the altitude (its distance above the sea floor) keeping system for an underwater robot. Visual recognition of distant underwater objects is possible in the water with high transparency, for example, in the coastal sea area of Okinawa prefecture, Japan. So, the authors have been adopting the distance measuring method using the two laser beams and a monocular camera with image processing. It realize to keep altitude of an underwater robot by using such devices. The evaluation experiments of the altitude keeping system are carried out in the pool.

Journal Articles

Temperature measurement of control rod using melt wire in High-Temperature Engineering Test Reactor (HTTR)

Hamamoto, Shimpei; Tochio, Daisuke; Ishii, Toshiaki; Sawahata, Hiroaki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 16(4), p.169 - 172, 2017/12

A melt wire was installed at the tip of the control rod in order to measure the temperature of High Temperature engineering Test Reactor (HTTR). After experience with reactor scrum from the state of reactor power 100%, the melt wire was taken out from the control rod and appearance has been observed visually. It was confirmed that the melt wires with a melting point of 505 $$^{circ}$$C or less were melted, and the melt wires with a melting point of 651 $$^{circ}$$C or more were not melted. Therefore, it was found that the highest arrival temperature of tip of the control rods where the melt wires are installed reaches within the range of 505 to 651 $$^{circ}$$C. And it was found that the control rod temperature at the time of reactor scram does not exceed the using temperature criteria (900 $$^{circ}$$C) of Alloy 800H of the control rod sleeve.

Journal Articles

Design and control of interface reaction between Al-based dielectrics and AlGaN Layer in AlGaN/GaN metal-oxide-semiconductor structures

Watanabe, Kenta*; Nozaki, Mikito*; Yamada, Takahiro*; Nakazawa, Satoshi*; Anda, Yoshiharu*; Ishida, Masahiro*; Ueda, Tetsuzo*; Yoshigoe, Akitaka; Hosoi, Takuji*; Shimura, Takayoshi*; et al.

Applied Physics Letters, 111(4), p.042102_1 - 042102_5, 2017/07

 Times Cited Count:16 Percentile:60.44(Physics, Applied)

AlGaN/GaN HFET (hetero-junction field-effect transitor) has gained much attention as next-generation high frequency and high power devices. In this study, we systematically investigated the interface reaction between Al-based dielectrics (Al$$_{2}$$O$$_{3}$$ and AlON) and AlGaN layer during deposition and post-deposition annealing (PDA), and revealed high thermal stability of AlON/AlGaN interface.

Journal Articles

A Recent experimental program to evidence in-vessel retention by controlled material relocation during core disruptive accidents of sodium-cooled fast reactors

Matsuba, Kenichi; Kamiyama, Kenji; Toyooka, Junichi; Zuev, V. A.*; Ganovichev, D. A.*; Kolodeshnikov, A. A.*

Proceedings of 10th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-10) (USB Flash Drive), 5 Pages, 2016/11

Molten fuel discharge through control rod guide tubes (CRGTs) is a key process that dominates the termination of core disruptive accidents of sodium-cooled fast reactors, since fuel dispersion from the core contributes to the achievement of both deeper subcriticality in the degraded core and formation of coolable debris bed. Within a framework of a collaborative research program between Japan Atomic Energy Agency and National Nuclear Center of the Republic of Kazakhstan, called EAGLE program, a new experimental program has been started with out-of-pile experiments to clarify the fuel discharge through CRGTs. This paper presents the status of the new program, including experimental results obtained so far.

Journal Articles

Level of detail control for environmental monitoring datasets

Miyamura, Hiroko; Takemiya, Hiroshi; Wu, H.-Y.*; Takahashi, Shigeo*

Kashika Joho Gakkai-Shi, 36(143), p.152 - 156, 2016/10

Broad survey on the distribution of the air dose rate has been performed after the accident at the Fukushima Daiichi Nuclear Power Plant continuously. The surveyed monitoring datasets are stored in a database and are made available to the public. Recently, the size of the datasets have been significantly increased as more detailed measurements in space and time are available, and effective reduction of the size of the datasets is necessary for visualizing and exploring such large scale datasets. However, if the datasets are not carefully reduced, we often miss a part of important features of the distribution data. Therefore, we develop an effective Level of Detail control (LoD) method for retaining critical features of the distribution. In the method, the global and local features of the distribution are extracted by means of differential topology analyses. Then, the simplified data is created by edge collapse operation with taking into account these features of the data.

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